بهینه‌سازی شرایط عملیاتی در یک سیستم اولترافیلتراسیون غشایی با استفاده از روش تاگوچی

نوع مقاله : مقاله پژوهشی

نویسندگان

1 پژوهشکده علوم و تکنولوژی پلیمر، پژوهشگاه صنعت نفت، تهران

2 دانشکده مهندسی شیمی و نفت، دانشگاه صنعتی شریف، تهران

چکیده

در این تحقیق، عملکرد یک غشای پلیمری تحت فرآیند اولترافیلتراسیون آب تولید شده همراه نفت با استفاده از یک فرآیند دو مرحله‌ای مورد بررسی قرار گرفت. در مرحله اول، تاثیر پارامترهای عملیاتی مانند اختلاف فشار دو طرف غشاء، دما و سرعت جریان عرضی خوراک بر روی میزان افت فلاکس ناشی از گرفتگی غشا در طول فرآیند مورد مطالعه قرار گرفت. برای طراحی آزمایشات و بهینه‌سازی نتایج آزمایشگاهی، از آرایه متعامد (33)9 L روش تاگوچی استفاده شد. برای تعیین مهم‌ترین پارامترهای موثر بر درصد افت فلاکس ناشی از گرفتگی غشاء، روش آنالیز واریانس مورد استفاده قرار گرفت. شرایط بهینه در سطح اول فشار (bar 5/1)، سطح دوم درجه حرارت (oC 40) و سطح سوم سرعت جریان عرضی (m/s 1) به دست آمد. در مرحله دوم، عملکرد سیستم اولترافیلتراسیون توسط غشای پلیمری تحت شرایط بهینه بررسی شد و میزان پس‌زنی روغن و گریس، TSS، کدورت و TOC به ترتیب برابر 99%، 100%، 99% و 68% دست آمد. همچنین اندازه ذرات موجود در خوراک از محدوده nm 800-200 به nm 3/0-5/1 کاهش یافت.
 

کلیدواژه‌ها


عنوان مقاله [English]

The Optimization of Operating Conditions in a Membrane Ultrafiltration System Using Taguchi Approach

نویسندگان [English]

  • Fatemeh Rekabdar 1
  • Ali Gheshlaghi 1
  • Mahmoud Hemmati 1
  • Amin Reyhani 2
  • forough Rajaei 2
1 Polymer Science and Technology Division, Research Institute of Petroleum Industry (RIPI)
2 Department of Chemical and Petroleum Engineering, Sharif University of Technology, Tehran
چکیده [English]

In this paper, the performance of a polymeric membrane was studied using a two-stage ultrafiltration treatment of produced water. At first, the effects of operating parameters, i.e. transmembrane pressure, temperature, and cross flow velocity on the flux decline caused by membrane fouling were investigated. In order to design the experiments and optimize the experimental results, the L9 (33) orthogonal array of Taguchi method was used. The analysis of variance was employed to determine the most significant parameters affecting the flux decline caused by membrane fouling. The optimum conditions were found at the first level of transmembrane pressure (1.5 bar), the second level of temperature (40 °C), and the third level of cross flow velocity (1 m/s). In the second stage, the performance of ultrafiltration system by the polymeric membrane was studied under the optimum conditions, 99% oil and grease, 100% TSS, 99% turbidity, and 68% TOC removal were obtained. Moreover, the particles size of the feed decreased from the range of 200-800 nm to 1.5-3 nm
 

کلیدواژه‌ها [English]

  • Produced Water
  • Ultrafiltration
  • Optimization
  • Taguchi
  • Polymeric Membrane
 
[1]. Asatekin A. and Mayes A. M., “Oil industry waste water treatment with fouling resistance membranes containing amphiphilic comb opolymers”, Environ. Sci. Technol., 43, 4487-4492, 2009.
[2]. Rezvanpour A., Roostaazad R., Hesampour M., Nystrom M., and Ghotbi C. , “Effective factors in the treatment of kerosene-water emulsion by using UF membranes”, J. Hazard. Mater., 161, 1216-1224, 2009.
[3]. Seo J. and Vogelpohl A. , “Membrane choice for waste water treatment using external cross flow tubular membrane filtration”, Desalination, 249, pp. 197-204, 2009.
[4]. Madaeni S. S., Gheshlaghi A. and Rekabdar F., “Membrane treatment of oily wastewater from refinery processes”, Asia-Pac. J. Chem. Eng., DOI: 10.1002/apj. pp. 1619, 2012.
[5]. Nouzaki K., Nagata J. and et al., “Preparation of polyacrynitrile ultrafiltration membranes for waste water treatment”, Desalination, 144, 53-59, 2002.
[6]. Gonder Z. B., Kaya Y., Vergili I. and Barlas H., “Optimization of filtration conditions for CIP wastewater treatment by nanofiltration process using Taguchi approach”, Sep. Purif. Technol., 70, 265-273, 2010.
[7] Schafer A. I., Fane A. G. and Waite T. D., Nanofiltration principles and applications, Elsevier Ltd., UK, 1-85617-405-0, 2005.
[8]. Falamaki C., Veysizadeh J., “Taguchi design of experiments approach to the manufacture of one-step alumina microfilter/membrane supports by the centrifugal casting technique”, Ceram. Int., 34, 1653–1659, 2008.
[9]. Peng W., I. Escobar C., White D. B., “Effects of water chemistries and properties of membrane on the performance and fouling-a model development study”, J. Membr. Sci., 238, 33–46, 2004.
[10]. Mousavi S. M., Yaghmaei S., Jafari A., Vossoughi M. and Ghobadi Z., “Optimization of ferrous biooxidation rate in a packed bed bioreactor using Taguchi approach”, Chem. Eng. Process., 46, 935–940, 2007.
[11]. Hesampour M., Kryzaniak A., Nystrom M., “The influence of different factors on the stability and ultrafiltration of emulsified oil in water”, J. Membr. Sci., 325, 199-208, 2008.
[12]. King S., Oily wastewater management study, Final Report, Cited at This Link:www.govlink.org/hazwaste, 1999.
[13]. Ross P. J., Taguchi techniques for quality engineering, 2nd ed., McGraw-Hill, New York, 1996.
[14]. Montgomery D. C., Design and analysis of experiments, (6th ed.), John Wiley & Sons, N.Y., 2005.
[15]. Masters I., Khoei A. R. and Gethin D. T., “The application of taguchi methods to the aluminum recycling process”, Proc. 4th ASM International Conference on the Recycling of Metals, Vienna, 115 – 124, 1991.
[16]. Janknecht P., Lopes D. and Mendes A. M., “Removal of industrial cutting oil from oil emulsions by polymeric ultra- and microfiltration membranes”, Environ. Sci. Technol., 38, 4878-4883, 2004.
[17]. Hesampour M., Kryzaniak A. and Nystorm M., “Treatment of waste water from metal working by ultrafiltration”, considering the effects of operating conditions, Desalination, 222, 212-221, 2008.
[18]. Sharma R. R., Agrawal R. and Chellam S., “Temperature effect on sieving characteristics of thin-film composite nanofiltration membranes: pore size distributions and transport parameters”, J. Membr. Sci., 223, 69–87, 2003.
[19]. Kowalska I., K. Majewska-Nowak, M. Kabsch-Korbutowicz, “Influence of temperature on anionic surface active agent removal from a water solution by ultrafiltration”, Desalination, 198, 124–131, 2006.
[20]. Mohammadi T. and Esmaeelifar A., “Wastewater treatment of a vegetable oil factory by a hybrid ultrafiltration-activated carbon process”, J. Membr. Sci., 54, 129-137, 2005.
[21]. Fernandez G., Carlos O., Carolina A., Garcia Y. and Mara S. L., The Study of Oil/Water Separation in Emulsion by Membrane Technology, SPE, Inc., 2001.
[22]. Banerjee P., DasGupta S., De S., “Removal of dye from aqueous solution using combination of advanced oxidation process and nanofiltration”, J. Hazard. Mater., 140, 95–103, 2007.
[23]. Abadi S. R. H., Sebzari M. R., Hemmati M., Rekabdar F. and Mohammadi T., “Ceramic membrane performance in microfiltration of oily wastewater”, Desalination, 265, 222–228, 2011.
[24]. Salahi A., Abbasi M. and Mohammadi T., “Permeate flux decline during UF of oily wastewater: Experimental and modeling”, Desalination, 251, 153–160, 2010.
[25]. Rahimpour A., Rajaeian B., Hosienzadeh A., Madaeni S. S. and Ghoreishi F., “Treatment of oily wastewater produced by washing of gasoline reserving tanks using self-made and commercial nanofiltration membranes”, Desalination, 265, 190–198, 2011.
[26]. Abbasi M., Sebzari M. R. and Mohammadi T., “Enhancement of Oily Wastewater Treatment by Ceramic Microfiltration Membranes using Powder Activated Carbon”, Chern. Eng. Technol., 34 (8), pp. 1252–1258, 2011.
[27]. Akdemir E. O., Ozer A., “Investigation of two ultrafiltration membranes for treatment of oily wastewater”, Desalination 249, pp. 660–666, 2009.